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Laurent PEDESSEAU

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Présentation

Education: ========== **2019:** Habilitation Degree in Physics, Université Rennes (France) **2004:** Ph.D in Physics, Université Paul Sabatier at Toulouse (France); Advisor: Prof. David Mainprice About: ====== Dr Pedesseau is an Associate Professor at the INSA Rennes (FOTON Institute - CNRS) whose work is aimed at the understanding of physical processes in the III-V semiconductor nanostructures for silicon photonics, the hybrid perovskites and novel materials for photovoltaics, and optoelectronic device simulations for optical-communications. His recent scientific interests include: 1) polar surface and interface energies of semiconductors; 2) first principles simulation (including the spin-orbit effect) of mechanical stability, electronic, and optical properties of 3D and 2D semiconductors; 3) electronic structure theory beyond the DFT such as hybrid functionals (HSE), many-body corrections GW, and DFT-1/2; 4) HPC technology for exotic and highly demanding simulations in terms of the large memory footprint and extensive CPUs communications (thousands). Employment: ============== **2011-present:** Associate Professor, Physics Department, INSA of Rennes, France **2008-2011:** Postdoctoral fellow, ICG and LCC, University of Montpellier, France **2006-2008:** Postdoctoral fellow, Physics Department, INSA of Rennes, France **2004-2006:** Postdoctoral fellow, Chemistry department, University College London, London, UK **2001-2004:** Ph.D. fellow, University Paul Sabatier, Toulouse, France Research interests: ====================== Material science, Semiconductor physics, Quantum nanostructures, Solar Energy, Advanced Materials Theoretical physics, Phase transitions, Dielectric and piezoelectric properties Density functional theory, k.p method, Finite element method Administrative responsibilities: =================================== **- Since 2016:** Leader of workgroup 1 (Nanostructure) for the COST Action MP1406 - MultiscaleSolar **- Since 2016:** In charge of International Affairs for the Materials science dept. at the INSA Rennes. Selected publications: ========================= \- Structural and thermodynamic limits of layer thickness in 2D halide perovskites. ***PNAS***, 116, 58, **2019** \- Concept of Lattice mismatch an emergence of surface states in 2D hybrid perovskite QW. ***Nano Lett.***, 18, 9, **2018** \- Universal description of III-V/Si epitaxial growth processes. ***Phys. Rev. Materials***, 2, 060401(R), **2018** \- A stress-free and textured GaP template on Si for sol. wat. split.. ***Ad. Funct. Mat.***, 28, 1801585, **2018** \- Scaling law for excitons in 2D perovskite quantum wells. ***Nat. Com.***, 9, 2254, **2018** \- Anharmonicity and Disorder in the Black Phases of etc. ***ACS Nano***, 12, 3477, **2018** \- Composite Nature of Layered Hybrid Perovskites: etc. ***ACS Nano***, 12, 3321, **2018** \- Hybrid Dion–Jacobson 2D Lead Iodide Perovskites. ***JACS***, 140, 3775, **2018** \- Decreasing the electronic confinement in layered perovskites through intercalation. ***Chem. Sci.***, **2017** \- Extremely efficient internal exciton dissociation through edge states in 2D HOP. ***Science***, 355, **2017** \- Advances and Promises of Layered Halide Hybrid Perovskite Semiconductors. ***ACS Nano***, 10, **2016** \- Rashba and Dresselhaus Effects in HOP: From Basics to Devices. ***ACS Nano***, 9, 11557, **2015** \- First-principles study of a NBS glass-former. I &II. ***Phys. Rev. B*** 91, 134201 & 134202, **2015** \- Analysis of Multivalley and Multibandgap Absorption etc. ***J. Phys. Chem. C*** 118, 11566, **2014** \- DFT and k·p modelling of the phase transitions of lead HOP etc. ***RRL*** 8, 31, **2014** \- Importance of soc in hop for photovoltaic applications. ***J. Phys. Chem. Lett.*** 4, 2999, **2013** \- Electronic model for self-assembled hybrid perovskite etc. ***Phys. Rev. B*** 86, 205301, **2012**

Publications

"antoine-letoublon"
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Study of MoS2 Deposited by ALD on c-Si, Towards the Development of MoS2/c-Si Heterojunction Photovoltaics

Bienlo Flora Zerbo , Mircea Modreanu , Ian Povey , Jun Lin , Antoine Létoublon
Crystals, 2022, 12 (10), pp.1363. ⟨10.3390/cryst12101363⟩
Article dans une revue hal-03792838v1
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Strong Electron–Phonon Interaction in 2D Vertical Homovalent III–V Singularities

Lipin Chen , Oliver Skibitzki , Laurent Pedesseau , Antoine Létoublon , Julie Stervinou
ACS Nano, 2020, 14 (10), pp.13127-13136. ⟨10.1021/acsnano.0c04702⟩
Article dans une revue hal-03032030v1

A study of the strain distribution by scanning X-ray diffraction on GaP/Si for III–V monolithic integration on silicon

Ang Zhou , Yanping Wang , Charles Cornet , Yoan Léger , Laurent Pedesseau
Journal of Applied Crystallography, 2019, 52 (4), pp.809-815. ⟨10.1107/S1600576719008537⟩
Article dans une revue hal-02289442v1
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A Stress-Free and Textured GaP Template on Silicon for Solar Water Splitting

Ida Lucci , Simon Charbonnier , Maxime Vallet , Pascal Turban , Yoan Léger
Advanced Functional Materials, 2018, 28 (30), pp.1801585. ⟨10.1002/adfm.201801585⟩
Article dans une revue hal-01803990v1
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Universal description of III-V/Si epitaxial growth processes

Ida Lucci , Simon Charbonnier , L. Pedesseau , Maxime Vallet , Laurent Cerutti
Physical Review Materials, 2018, 2 (6), pp.060401(R). ⟨10.1103/PhysRevMaterials.2.060401⟩
Article dans une revue hal-01833206v1
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Monolithic Integration of Diluted-Nitride III–V-N Compounds on Silicon Substrates: Toward the III–V/Si Concentrated Photovoltaics

Olivier Durand , Samy Almosni , Yanping Wang , C. Cornet , A. Létoublon
Energy Harvesting and Systems, 2014, 1 (3-4), pp.147-156. ⟨10.1515/ehs-2014-0008⟩
Article dans une revue hal-01166477v1
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Structural and optical properties of (In,Ga)As/GaP quantum dots and (GaAsPN/GaPN) diluted-nitride nanolayers coherently grown onto GaP and Si substrates for photonics and photovoltaics applications

Olivier Durand , Cédric Robert Robert , Thanh Tra Nguyen , Samy Almosni , Thomas Quinci
Proceedings of SPIE, the International Society for Optical Engineering, 2013, Quantum sensing and nanophotonic devices X, 8631, pp.863126. ⟨10.1117/12.2012670⟩
Article dans une revue hal-00842763v1

Evaluation of InGaPN and GaAsPN materials lattice-matched to Si for multi-junction solar cells

Samy Almosni , Cédric Robert Robert , Thanh Tra Nguyen , Charles Cornet , Antoine Létoublon
Journal of Applied Physics, 2013, 113 (12), pp.123509. ⟨10.1063/1.4798363⟩
Article dans une revue hal-00918663v1

Light emitting diodes on silicon substrates: preliminary results

Alexandre Bondi , Weiming Guo , Laurent Pedesseau , Soline Boyer-Richard , Hervé Folliot
physica status solidi (c), 2009, 6 (10), pp.2212-2216. ⟨10.1002/PSSC.200881728⟩
Article dans une revue hal-00665750v1

Optical and structural characterization of thin MoS2 layers on SiO2/Si substrates, towards the development of MoS2/Si heterojunction photovoltaics.

Bienlo Flora Zerbo , Mircea Modreanu , Ian Povey , Antoine Letoublon , Alain Rolland
44th International Semiconductor Conference (CAS 2021), Oct 2021, Online, Romania. ⟨10.1109/CAS52836.2021.9604140⟩
Communication dans un congrès hal-03796793v1

GaPSb/Si tandem material with APBs for efficient overall water splitting

Lipin Chen , Mahdi Alqahtani , Christophe Levallois , Antoine Létoublon , Julie Le Pouliquen
Journées Nanomatériaux de Rennes, Jan 2020, Rennes, France
Communication dans un congrès hal-03032905v1

Solar Water Splitting: surface energy engineering of GaP Template on Si

Laurent Pedesseau , Ida Lucci , Simon Charbonnier , Pascal Turban , Yoan Léger
European Materials Research Society - Spring Meeting 2019 (E-MRS 2019 Spring Meeting), Apr 2019, Phoenix, United States
Communication dans un congrès hal-02114792v1

GaPSb/Si photoelectrode for Solar Fuel Production

Lipin Chen , Christophe Levallois , Antoine Létoublon , Julie Le Pouliquen , Rozenn Piron
European COST multsicaleSolar Final meeting, Apr 2019, Sofia, Bulgaria
Communication dans un congrès hal-03102622v1

III-V/Si photoelectrodes: a new route for solar hydrogen production

Charles Cornet , Lipin Chen , Mahdi Alqahtani , Christophe Levallois , Antoine Létoublon
11è Journées Scientifiques de Porquerolles (JSP2019), C'Nano-PACA, Sep 2019, Porquerolles, France
Communication dans un congrès hal-02305423v1

A universal mechanism to describe III-V epitaxy on Si

Ida Lucci , Simon Charbonnier , Laurent Pedesseau , Maxime Vallet , Laurent Cerutti
20th European Molecular Beam Epitaxy Workshop (Euro-MBE 2019), Feb 2019, Lenggries, Germany
Communication dans un congrès hal-02048639v1

Universal growth mechanism of III-V/Si: using antiphase boundaries for devices.

Charles Cornet , Ida Lucci , Lipin Chen , Laurent Pedesseau , Rozenn Bernard
Réunion plénière du GDR Pulse (PULSE 2019), Jul 2019, Clermont-Ferrand, France
Communication dans un congrès hal-02189095v1

(114) GaP surface texturation on Si for water splitting

Ida Lucci , Simon Charbonnier , Maxime Vallet , Pascal Turban , Yoan Léger
EMRS Spring meeting 2018, Jun 2018, Strasbourg, France
Communication dans un congrès hal-01708047v1

A general III-V/Si growth process description

Ida Lucci , Simon Charbonnier , Laurent Pedesseau , Maxime Vallet , Laurent Cerutti
European Materials Research Society - Spring Meeting 2018 (E-MRS 2018 Spring Meeting), Jun 2018, Strasbourg, France
Communication dans un congrès hal-01910535v1

III-V/Si heterogeneous growth : thermodynamics and antiphase domains formation

Ida Lucci , Simon Charbonnier , Laurent Pedesseau , Maxime Vallet , Laurent Cerutti
34th International Conference on the Physics of Semiconductors (ICPS 2018), Jul 2018, Montpellier, France
Communication dans un congrès hal-01910543v1

GaP Template on Si for Solar Water Splitting: surface energy engineering

Laurent Pedesseau , Ida Lucci , Simon Charbonnier , Maxime Vallet , Pascal Turban
nanoGe Fall Meeting 2018 (NGFM18), Oct 2018, Torremolinos, Spain
Communication dans un congrès hal-01909068v1

A universal mechanism to describe the III-V on Si growth by Molecular Beam Epitaxy

Ida Lucci , Simon Charbonnier , Laurent Pedesseau , Maxime Vallet , Laurent Cerutti
20th International Conference on Molecular-Beam Epitaxy (ICMBE 2018), Sep 2018, Shanghai, China. pp.Th-C1-3(S)
Communication dans un congrès hal-01910554v1

Large scale textured GaP(114) growth on vicinal Si substrate by Molecular Beam Epitaxy for water splitting applications

Ida Lucci , Simon Charbonnier , Maxime Vallet , Pascal Turban , Yoan Léger
20th International Conference on Molecular-Beam Epitaxy (ICMBE 2018), Sep 2018, Shanghai, China. pp.Tu-P-43(S)
Communication dans un congrès hal-01910556v1

Nano Beam X-ray Scattering on GaP/Si for III-V Monolithic Integration on Silicon

Ang Zhou , Yanping Wang , Antoine Létoublon , Ida Lucci , Charles Cornet
European Materials Research Society - Spring Meeting 2018 (E-MRS 2018 Spring Meeting), Jun 2018, Strasbourg, France
Communication dans un congrès hal-02352639v1

III-V/Si 3D crystal growth: a thermodynamic description

Ida Lucci , Simon Charbonnier , Maxime Vallet , Tony Rohel , Rozenn Bernard
Energy Materials Nanotechnology Meeting 2017 / Collaborative Conference on Crystal Growth (EMN 3CG 2017), Aug 2017, Berlin, Germany
Communication dans un congrès hal-01708282v1

GaP/Si(001) polar-on-nonpolar epitaxial growth revisited by scanning tunneling microscopy.

Simon Charbonnier , Ida Lucci , Subhashis Gangopadhyay , Yanping Wang , Tony Rohel
Réunion plénière du GDR Pulse (PULSE 2017), Oct 2017, Paris, France
Communication dans un congrès hal-01715954v1

GaP/Si(001) polar-on-nonpolar epitaxial growth revisited by scanning tunneling microscopy

Simon Charbonnier , Ida Lucci , Subhashis Gangopadhyay , Yanping Wang , Tony Rohel
16th International Conference on the Formation of Semiconductor Interfaces (ICFSI-16), Jul 2017, Hannover, Germany
Communication dans un congrès hal-01715971v1

3D GaP/Si(001) growth mode and antiphase boundaries

Ida Lucci , Simon Charbonnier , Yanping Wang , M. Bahri , Maxime Vallet
19th International Conference on Molecular-Beam Epitaxy (IC-MBE 2016), Sep 2016, Montpellier, France
Communication dans un congrès hal-01497144v1

Etude de la croissance cohérente de GaP/Si(001) en couche mince

Ida Lucci , Simon Charbonnier , Yanping Wang , Mounib Bahri , Maxime Vallet
Réunion plénière du GDR Pulse (PULSE 2016), Jul 2016, Marseille, France
Communication dans un congrès hal-01497149v1

First stage results on III-V/Si tandem cells using GaAsPN dilute-nitride

Mickael da Silva , Charles Cornet , Antoine Létoublon , Christophe Levallois , Alain Rolland
European Materials Research Society - Spring Meeting 2016 (E-MRS 2016 Spring Meeting), May 2016, Lille, France
Communication dans un congrès hal-01496924v1

Advanced concepts of photovoltaics based on III-V compounds

Olivier Durand , Mickael da Silva , Yanping Wang , Charles Cornet , Antoine Létoublon
16th International Conference of Physical Chemistry (ROMPHYSCHEM-16), Sep 2016, Galaţi, Romania
Communication dans un congrès hal-01496667v1

Quantitative evaluation of microtwins and antiphase defects towards a GaP/Si platform for monolithic integrated photonics

Yanping Wang , Antoine Létoublon , Thanh Tra Nguyen , G. Patriarche , Anne Ponchet
European Materials Research Society - Spring Meeting 2015 (E-MRS 2015 Spring Meeting), May 2015, Lille, France
Communication dans un congrès hal-01497220v1

Numerical and experimental ongoing on III-V/Si high-efficiency tandem solar cell

Mickael da Silva , Shijian Wang , Samy Almosni , Charles Cornet , Antoine Létoublon
European Congress and Exhibition on Advanced Materials and Processes (EUROMAT 2015), Sep 2015, Warsaw, Poland
Communication dans un congrès hal-01203374v1

Toward the III-V/Si high efficiency tandem solar cell

Olivier Durand , Samy Almosni , Mickael da Silva , Charles Cornet , Antoine Létoublon
7th International Workshop on "Advanced optical and X-ray characterization techniques of multifunctional materials for information and communication technologies, health and renewable energy applications", Sep 2015, Bucarest, Romania
Communication dans un congrès hal-01497190v1

Epitaxie cohérente de composés GaP et GaAsPN à azote dilué sur substrats de Si pour l’élaboration de cellules PV tandem III-V/Si

Olivier Durand , Samy Almosni , Yanping Wang , Charles Cornet , Antoine Létoublon
Matériaux 2014, Nov 2014, Montpellier, France
Communication dans un congrès hal-01115312v1

Ab initio investigation of defect nucleation at III-V/Si heterointerface for tandem solar cells applications

Eric Tea , Charles Cornet , Antoine Létoublon , J. Vidal , Laurent Pedesseau
European Materials Research Society meeting E-MRS 2013, May 2013, Strasbourg, France
Communication dans un congrès hal-00918729v1

Monolithic integration of diluted-nitride III-V-N compounds on silicon substrates : toward the III-V/Si Concentrated Photovoltaics

Olivier Durand , Samy Almosni , Cédric Robert Robert , Thanh Tra Nguyen , Yanping Wang
International Symposium on Inorganic and Environmental Materials, Oct 2013, Rennes, France
Communication dans un congrès hal-00918754v1

Monolithic growth of III-V-N diluted nitride devices on Si substrate for solar cells

Olivier Durand , Samy Almosni , Cédric Robert Robert , Thanh Tra Nguyen , Charles Cornet
Journées nationales du photovoltaïque JNPV2012, 2012, Chantilly, France
Communication dans un congrès hal-00788544v1

Raman investigation of GaP-Si interfaces grown by molecular beam epitaxy

Alexandre Bondi , Charles Cornet , Soline Richard , Thanh Tra Nguyen , Antoine Létoublon
European Materials Research Society Spring Meeting 2012 (E-MRS Spring 2012), May 2012, Strasbourg, France. pp.72-75, ⟨10.1016/j.tsf.2012.11.132⟩
Communication dans un congrès hal-00788308v1

Stransky-Krastanow Gas Source MBE growth and optical properties of InAs/GaP quantum dots

Charles Cornet , Olivier Dehaese , Laurent Pedesseau , Ibrahim Alghoraibi , Tony Rohel
euro-MBE conference, Mar 2007, Sierra nevada, Granada, France. pp.1
Communication dans un congrès hal-00491810v1

Performances of III-P/Si based photoelectrodes for solar hydrogen production

Lipin Chen , Mekan Piriyev , Antoine Létoublon , Olivier Durand , Laurent Pedesseau
Journées Nationales du photovoltaïque 2020, Jan 2021, Dourdan, France. 2021
Poster de conférence hal-03032889v1

Electron-phonon interactions around antiphase boundaries in InGaP/SiGe/Si : structural and optical characterizations

Lipin Chen , Rozenn Piron , Oliver Skibitzki , Yoan Léger , Christophe Levallois
International Symposium : 20th Anniversary of LPQM, Apr 2019, Cachan, France
Poster de conférence hal-02882424v1

A Study on the Strain Distribution by Scanning X-ray diffraction on GaP/Si for III-V Monolithic Integration on Silicon for Nonlinear Optics

Ang Zhou , Yanping Wang , Charles Cornet , Yoan Léger , Laurent Pedesseau
Rayons X et Matière 2019, Nov 2019, Nancy, France
Poster de conférence hal-03108397v1

Study of the 3D growth mode of III-V on Si by DFT

Ida Lucci , Simon Charbonnier , Yanping Wang , Tony Rohel , Rozenn Bernard
Réunion plénière du GDR Pulse (PULSE 2017), Oct 2017, Paris, France
Poster de conférence hal-01708149v1
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Towards III-V on silicon solar cells

Mickael da Silva , S. Boyer-Richard , C. Cornet , Antoine Létoublon , Christophe Levallois
7è Journées Nationales du PhotoVoltaïque (JNPV 2017), Dec 2017, Dourdan, France. 107, pp.191603 - 191603, 2015
Poster de conférence hal-01660154v1
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X-ray Coherent Scattering on GaP/Si for III-V Monolithic Integration on Silicon

Yanping Wang , Antoine Létoublon , Ida Lucci , Charles Cornet , V. Favre-Nicolin
International Workshop on Phase Retrieval and Coherent Scattering (COHERENCE 2016), Jun 2016, Saint-Malo, France. 2016
Poster de conférence hal-01496666v1

Relationship between antiphase domains, roughness and surface/interface energies during the epitaxial growth of GaP on Si

Ida Lucci , Simon Charbonnier , Yanping Wang , Mounib Bahri , Maxime Vallet
European Materials Research Society - Spring Meeting 2016 (E-MRS 2016 Spring Meeting), May 2016, Lille, France
Poster de conférence hal-01497064v1

GaAsPN Single and Tandem Solar Cells on Silicon

Mickael da Silva , Charles Cornet , Antoine Létoublon , Christophe Levallois , Alain Rolland
19th International Conference on Molecular-Beam Epitaxy (IC-MBE 2016), Sep 2016, Montpellier, France
Poster de conférence hal-01496922v1

Vers les cellules solaires à haut rendement à base de composés III-V sur substrats bas-couts de silicium

Mickael da Silva , Samy Almosni , Charles Cornet , Antoine Létoublon , Christophe Levallois
Optique Bretagne 2015 - Horizons de l'Optique, Jul 2015, Rennes, France
Poster de conférence hal-01497238v1